By A. F. Andresen
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Additional info for Hydrides for Energy Storage. Proceedings of an International Symposium Held in Geilo, Norway, 14–19 August 1977
Example text
However, in some metallic hosts the energetics are unfavorable for total occupancy of a particular set of interstitial sites and only partial occupancy occurs. This gives rise to arrangements that are not structurally unique and the possibility of order-disorder transformations involving the occupied and unoccupied sites, features which confer structural complexity on these kinds of metallic hydrides. Some of these complexities have been revealed in detailed studies of Ta H and are elaborated upon in a later section of this paper.
Other Alkaline earths (half of the hydrogen) ; rare earth trihydrides (one-third of the hydrogen) J a. b. c. d. e. f. g. h. i. j. Ref. 3 J. E. , M. K. Wilkinson and C. G. Shull, J. Phys. Chem. Solids 3_, 303 (1957). J. W. Cable, E. 0. Wollan and W. C. Koehler, Int. Colloquium on Diffraction and Diffusion of Neutrons, CHRS Publ. No. 12t (1964), p. 36. Ref. 4 D. E. Cox, G. Shirane, W. J. Takei and W. E. Wallace, J. Appl. Phys. , 1342 (1963) and C. E. Holley, R. N. R. Mulford, F. H. Ellinger, W. C.
Similar considerations hold for Y b 3 + ; it captures a conduction electron to achieve a filled 4f shell. The limiting stoichiometries of Eu and Yb hydrides and their structures strongly support the view that these are saline hydrides, stabilized primarily by ionic bonding, and hence they should be represent ed as R 2 + ( H ~ ) 2 where R = Eu or Yb. TRANSITION METAL HYDRIDES Early Pd-H Studies - The Birth of the Protonic Model Extensive hydride formation is exhibited by metals in the titanium and vanadium groups.
